Pierre Curie, Recent research on radioactivity (1904)
“ When one wishes to excite a solid to saturation with the emanation from thorium, it is necessary to cause the emanation to act for a long time, and hence new supplies of it must be brought continually to the surface of the body that is to be excited. To do this a current of air is passed through a solution of a salt of thorium and, then this current, of air charged with the emanation, is passed over the body. The solid, when excited by the emanation from thorium, loses its activity spontaneously according to an exponential law. The radiation falls to one-half every eleven hours. ”
