Pierre Curie, Recent research on radioactivity (1904)
“ It loses one-half of its value every four days. To interpret this phenomenon it must be assumed that radium continuously gives off a constant radioactive emanation. This emanation spreads into the air in a closed space, and acting on solids, makes them radioactive. When the air is transferred to another space, the emanation is carried along with it. Finally, it is destroyed spontaneously with such velocity that the quantity of emanation in the gas diminishes by one-half every four days. ”
